Simultaneous manipulation of iron(ii) spin crossover and LIESST behaviour using pressure, temperature and light

Autor(en)
Gabriela Handzlik, Kamil F. Dziubek, Michael Hanfland, Dawid Pinkowicz
Abstrakt

Spin crossover (SCO) and light-induced excited spin state trapping (LIESST) effects were studied using high pressure X-ray diffraction at cryogenic temperatures on a single crystal of the {[FeII(pyrazole)4]2[NbIV(CN)8]·4H2O}n (FeNb) coordination polymer. The studied compound does not show SCO or LIESST at ambient pressure, but these effects can be enforced by a mechanical stimulus. The obtained results demonstrate the manipulation of the spin state via the appropriate combination of multiple stimuli simultaneously.

Organisation(en)
Institut für Mineralogie und Kristallographie
Externe Organisation(en)
Jagiellonian University in Krakow, European Synchrotron Radiation Facility ESRF
Journal
Dalton Transactions
Band
53
Seiten
7677-7681
Anzahl der Seiten
5
ISSN
1477-9226
DOI
https://doi.org/10.1039/d4dt00509k
Publikationsdatum
04-2024
Peer-reviewed
Ja
ÖFOS 2012
105113 Kristallographie, 104003 Anorganische Chemie, 104017 Physikalische Chemie, 104011 Materialchemie
Schlagwörter
ASJC Scopus Sachgebiete
Inorganic Chemistry
Link zum Portal
https://ucrisportal.univie.ac.at/de/publications/2891da47-5a2e-4c11-a654-6ad8d9895ab8