X-ray structural study of intermetallic alloys RT2Si and RTSi2 (R=rare earth, T=noble metal)

Autor(en)
Alexander V Gribanov, Andrij Grytsiv, Peter Franz Rogl, Yuri D. Seropegin, Gerald Giester
Abstrakt

Two series of intermetallic alloys, RT 2Si and RTSi2, have been synthesized from stoichiometric compns. The crystal structures of EuPt1+ xSi2- x (CeNiSi2-type), CeIr2Si (new structure type), YbPd2Si and YbPt2Si (both YPd2Si-type) have been elucidated from X-ray single crystal CCD data, which were confirmed by XPD expts. The crystal structures of LaRh2Si and LaIr2Si (CeIr2Si-type), {La,Ce,Pr,Nd}AgSi2 (all TbFeSi2-type), and EuPt2Si (inverse CeNiSi2-type) were characterized by XPD data. RT 2Si/RTSi2 compds. were neither detected in as-cast alloys Sc25Pt50Si25, Eu25Os25Si50 and Eu25Rh25Si50 nor after annealing at 900 C. Instead, X-ray single crystal data prompted Eu2Os3Si5 (Sc2Fe3Si5-type) and EuRh2+ xSi2- x (x=0.04, ThCr2Si2-type) as well as a new structure type for Sc2Pt3Si2 (own type).

Organisation(en)
Institut für Physikalische Chemie, Institut für Mineralogie und Kristallographie
Externe Organisation(en)
Lomonosov Moscow State University (MSU)
Journal
Journal of Solid State Chemistry
Band
183
Seiten
1278-1289
Anzahl der Seiten
12
ISSN
0022-4596
DOI
https://doi.org/10.1016/j.jssc.2010.03.038
Publikationsdatum
2010
Peer-reviewed
Ja
ÖFOS 2012
104017 Physikalische Chemie, 105113 Kristallographie
Link zum Portal
https://ucrisportal.univie.ac.at/de/publications/4484bfa9-bc8b-402b-958b-79c7a7285ae8