Sodium-potassium interdiffusion in potassium-rich alkali feldspar II

Autor(en)
Anne-Kathrin Schäffer, Elena Petrishcheva, Gerlinde Habler, Rainer Abart, Dieter Rhede, Gerald Giester
Abstrakt

Na-K interdiffusion in disordered potassium-rich alkali feldspar was studied experimentally using cation exchange between gem quality sanidine from the Eifel and alkali-halide melt at temperatures of 800 °C to 1000 °C and at close to ambient pressure. Sodium-potassium interdiffusion coefficient DNaK was determined for potassium mole fractions in the range 0.65 < XOr < 0.99. At 0.65 < XOr < 0.95 the sodium-potassium interdiffusion coefficient is largely independent of composition. At XOr > 0.95, it rises sharply with increasing potassium mole fraction. Diffusion perpendicular to (001) is about one order of magnitude faster and less strongly temperature dependent than perpendicular to (010). The parameters of the Arrhenius equation describing the temperature dependence of the sodium-potassium interdiffusion coefficient DNaK D0Exp (EA/RT) were estimated as D0 (001)(0.92) 5.18 108 m2/s, EA (001)(0.92) 179kJ/mole D0 (001)(0.98) 1.82 107 m2/s, EA (001)(0.98) 182kJ/mole D0 (010)(0.92) 5.81 105 m2/s, EA (010)(0.92) 272kJ/mole D0 (010)(0.98) 1.34 104 m2/s, EA (010)(0.98) 269kJ/mole. The results of our direct determinations are compared with theoretical calculations using the corresponding sodium- and potassium tracer-diffusion coefficients, and the processes underlying the observed composition- and temperature dependence of sodium-potassium interdiffusion are discussed.

Organisation(en)
Department für Lithosphärenforschung, Institut für Mineralogie und Kristallographie
Externe Organisation(en)
Helmholtz-Zentrum Potsdam Deutsches GeoForschungsZentrum
Journal
American Journal of Science: an international earth science journal
Band
314
Seiten
1300-1318
Anzahl der Seiten
19
ISSN
0002-9599
DOI
https://doi.org/10.2475/09.2014.03
Publikationsdatum
11-2014
Peer-reviewed
Ja
ÖFOS 2012
105116 Mineralogie, 105113 Kristallographie, 105120 Petrologie
Schlagwörter
ASJC Scopus Sachgebiete
Allgemeine Erdkunde und Planetologie
Link zum Portal
https://ucrisportal.univie.ac.at/de/publications/7a49776e-79d1-440d-83cd-1adab6c1de02