Tschörtnerite, a copper-bearing zeolite from Bellberg volcano, Eifel, Germany

Autor(en)
Herta Silvia Effenberger, Gerald Giester, Werner Krause, Heinz-Jürgen Bernhardt
Abstrakt

The new mineral tschortnerite, ideally Ca4(K,Ca,Sr,Ba)3Cu3(OH)8[Al12Si12O48]×xH2O, x ³ 20, occurs as well-formed cubes up to a max. size of 0.15 mm in a Ca-rich xenolith at the Bellberg volcano near Mayen, Eifel, Germany. The light blue, transparent crystals are optically isotropic, n = 1.504(2). Microprobe anal. (in wt. percent) gave CaO 13.10, CuO 9.64, SrO 4.49, BaO 1.93 K2O 1.37, Fe2O3 0.30, Al2O3 25.21, SiO2 30.25, H2O (calc. by difference) 13.71. The empirical formula based on 48 O atoms within the tetrahedral net is Ca5.60Sr1.04K0.70Ba0.30Cu2.90Fe0.09Al11.85Si12.06O48(OH)8.44×14.01H2O. Tschortnerite is cubic, space group Fm.hivin.3m [a = 31.62(1) .ANG., V = 31614 .ANG.3, Z = 16]. The d. is Dmeas = 2.1 g/cm3, Dcalc = 2.10 g/cm3. Single-crystal X-ray investigations showed that tschortnerite is a zeolite; the structure contains interconnection of double six-rings, double eight-rings, sodalite cages, truncated cubo-octahedra, and previously unknown 96-membered cages (tschortnerite cage). A new structural unit is the [Cu12(OH)24]Ca8O24(H2O)8 cluster centered within the truncated cubo-octahedron. The cluster is formed by a rhomb-dodecahedron-like arrangement of corner connected CuO4 squares, the eight CaO7 polyhedra are branched. The sodalite cage houses Ca4(OH)4O12 clusters of edge-sharing CaO6 octahedra. Half-occupied (K,Ca,Sr,Ba) positions were located in the basal and top face of the double eight-rings, i.e., the border to the tschortnerite cage. Within the large tschortnerite cage only H2O mols. were localized.

Organisation(en)
Institut für Mineralogie und Kristallographie
Externe Organisation(en)
Ruhr-Universität Bochum (RUB)
Journal
The American mineralogist
Band
83
Seiten
607-617
Anzahl der Seiten
11
ISSN
0003-004X
DOI
https://doi.org/10.2138/am-1998-5-620
Publikationsdatum
06-1998
Peer-reviewed
Ja
ÖFOS 2012
105113 Kristallographie, 105116 Mineralogie
Link zum Portal
https://ucrisportal.univie.ac.at/de/publications/tschoertnerite-a-copperbearing-zeolite-from-bellberg-volcano-eifel-germany(e4ae3959-e036-4b38-a584-3243a2b19125).html