Tourmaline of the elbaite-schorl series from the Himalaya Mine, Mesa Grande, California: A detailed investigation

Autor(en)
Andreas Ertl, George R. Rossman, John M. Hughes, David London, Ying Wang, Julie A. O'Leary, M. Darby Dyar, Stefan Prowatke, Thomas Ludwig, Ekkehart Tillmanns
Abstrakt

Chemical, structural, infrared, optical, and Mössbauer spectroscopic data were obtained on tourmalines from gem pockets in the Himalaya mine, San Diego County, California, including a strongly color-zoned crystal. Calcium and Li abundances increase from core to rim, whereas Mn2+ and F increase, reach a maximum, and then decrease. Upon initiation of crystallization of lepidolite, F contents in tourmaline decrease. The black core is a Mn-bearing "oxy-schorl." The grayish-yellow, intermediate zone is Mn-rich "fluor-elbaite" that contains a relatively high Mn content with ~6 wt% MnO. The nearly colorless "fluor-elbaite" rim has the highest Li content of all zones. There is an inverse correlation between the lattice parameter a (for values =15.84 Å) and the Li content (r2 = 0.96). Mössbauer studies from the different zones within this crystal show that the Fe3+/Fe(total) ratio increases continuously from the Fe-rich core to the Fe-poor near-rim zone, consistent with increasing oxygen fugacity during pegmatite pocket evolution. There is a high positive correlation between lat¬tice parameter a (for values =15.84 Å) and (Fe2++Mn2+) content in tourmalines from the elbaite-schorl series (r2 = 0.99). Values lower than 15.84 Å for a are likely a consequence of greater [4]B contents in samples that usually have a (Fe2++Mn2+) content of

Organisation(en)
Institut für Mineralogie und Kristallographie
Externe Organisation(en)
California Institute of Technology (Caltech), Miami University, University of Oklahoma, Universität Heidelberg, Mount Holyoke College
Journal
American Mineralogist: an international journal of earth and planetary materials
Band
95
Seiten
24-40
Anzahl der Seiten
17
ISSN
0003-004X
DOI
https://doi.org/10.2138/am.2010.3271
Publikationsdatum
2010
Peer-reviewed
Ja
ÖFOS 2012
105113 Kristallographie, 105116 Mineralogie
Link zum Portal
https://ucrisportal.univie.ac.at/de/publications/ef47d286-1556-46af-aec0-88bf342b1c74