Simultaneous manipulation of iron(ii) spin crossover and LIESST behaviour using pressure, temperature and light

Author(s)
Gabriela Handzlik, Kamil F. Dziubek, Michael Hanfland, Dawid Pinkowicz
Abstract

Spin crossover (SCO) and light-induced excited spin state trapping (LIESST) effects were studied using high pressure X-ray diffraction at cryogenic temperatures on a single crystal of the {[FeII(pyrazole)4]2[NbIV(CN)8]·4H2O}n (FeNb) coordination polymer. The studied compound does not show SCO or LIESST at ambient pressure, but these effects can be enforced by a mechanical stimulus. The obtained results demonstrate the manipulation of the spin state via the appropriate combination of multiple stimuli simultaneously.

Organisation(s)
Department of Mineralogy and Crystallography
External organisation(s)
Jagiellonian University in Krakow, European Synchrotron Radiation Facility ESRF
Journal
Dalton Transactions
Volume
53
Pages
7677-7681
No. of pages
5
ISSN
1477-9226
DOI
https://doi.org/10.1039/d4dt00509k
Publication date
04-2024
Peer reviewed
Yes
Austrian Fields of Science 2012
105113 Crystallography, 104003 Inorganic chemistry, 104017 Physical chemistry, 104011 Materials chemistry
Keywords
ASJC Scopus subject areas
Inorganic Chemistry
Portal url
https://ucrisportal.univie.ac.at/en/publications/2891da47-5a2e-4c11-a654-6ad8d9895ab8