Crystal structures, site occupations and phase equilibria in the system V-Zr-Ge

Author(s)
Martin Marker, Herta Silvia Effenberger, Klaus Richter
Abstract

The V-Zr-Ge system was studied for two isothermal sections at 900 and 1200 °C. Three ternary compounds VZrGe (tI12, I4/mmm, CeScSi-type), VxZr5-xGe4 (oP36, Pnma, Sm5Ge4-type) and V4+xZr2-xGe5 (oI44, Ibam, Si5V6-type) were structurally characterized. Optical microscopy and powder X-ray diffraction (XRD) were used for initial sample characterization and electron probe microanalysis (EPMA) of the annealed samples was used to determine the exact phase compositions. The variation of the cell parameters of the various ternary solid solutions with the composition was determined. The three ternary phases were structurally characterized by means of single crystal and powder XRD. While VZrGe is almost a line compound, VxZr5-xGe4 (0.2 ? x ? 3.0) and V4+xZr2-xGe5 (0.06 ? x ? 1.2) are forming extended solid solution ranges stabilized by differential fractional site occupancy of V and Zr on the metal sites.

Organisation(s)
Department of Functional Materials and Catalysis, Department of Mineralogy and Crystallography
Journal
Solid State Sciences
Volume
11
Pages
1475-1483
No. of pages
9
ISSN
1293-2558
DOI
https://doi.org/10.1016/j.solidstatesciences.2009.05.005
Publication date
2009
Peer reviewed
Yes
Austrian Fields of Science 2012
104003 Inorganic chemistry, 105113 Crystallography, 104011 Materials chemistry
Portal url
https://ucrisportal.univie.ac.at/en/publications/450c7349-c3ad-4c55-8e08-7b4e23e93f05