Synthesis, crystal structure and antibacterial activities of mixed ligand copper(II) and cobalt(II) complexes of a NNS Schiff base

Author(s)
Mahendra Ghosh, Manas Layek, Michel Fleck, Rajat Saha, Debasis Bandyopadhyay
Abstract

Two new copper(II) complexes of different nuclearities, viz. mononuclear [CuL2(H2O)](ClO4)2 (1), binuclear [Cu2L2(NCS)2(NO3)2] (2) and a mononuclear cobalt(II) complex, [CoL2(NCS)2] (3), where HL = 2-{[pyridin-2-ylmethylidene]amino}benzenethiol, a tridentate Schiff base derived from 2-aminothiophenol and pyridine-2-al have been prepd. The complexes have been characterized by microanal., spectroscopic, single crystal X-ray diffraction and other physicochem. studies. Structural studies reveal that 1 is a mononuclear copper(II) complex with distorted square pyramidal geometry. But, 2 is a thiocyanato-bridged binuclear species in which each copper(II) ion adopts an irregular octahedral geometry contg. chelating nitro groups. Complex 3 is comprised of a mononuclear octahedral unit contg. two thiocyanato groups in cis positions around the central cobalt(II) ion. The complex units in 1-3 are held together by H-bonding, p···p or O···p interactions to develop supramol. network in their resp. solid states. The antibacterial activity of all the complexes along with the constituent Schiff base ligand has been evaluated against some Gram(+) and Gram(-?) bacteria.

Organisation(s)
Department of Mineralogy and Crystallography
External organisation(s)
Bankura Christian College, Jadavpur University
Journal
Polyhedron
Volume
85
Pages
312-319
No. of pages
8
ISSN
0277-5387
DOI
https://doi.org/10.1016/j.poly.2014.08.014
Publication date
08-2014
Peer reviewed
Yes
Austrian Fields of Science 2012
104015 Organic chemistry, 104011 Materials chemistry, 105113 Crystallography, 301206 Pharmacology
Keywords
ASJC Scopus subject areas
Materials Chemistry, Inorganic Chemistry, Physical and Theoretical Chemistry
Portal url
https://ucrisportal.univie.ac.at/en/publications/synthesis-crystal-structure-and-antibacterial-activities-of-mixed-ligand-copperii-and-cobaltii-complexes-of-a-nns-schiff-base(d34def5f-b1a2-4e9a-8358-f42367b39641).html