A Discrete Chloride Monohydrate

Author(s)
Mohammed S. Abdelbassit, Owen J. Curnow, Eugen Libowitzky, Ross O. Piltz, Matthew I. J. Polson
Abstract

The solid-state structure of a discrete chloride monohydrate species, [Cl(H2O)]-, is reported for the first time. It was isolated as a salt of the tris(dipropylamino)cyclopropenium cation and has been structurally characterized by X-ray and neutron diffraction. Infrared (IR), far-infrared, and Raman spectroscopic studies were also carried out. Additionally, the D2O and HDO isotopomers were investigated. Of the six fundamental vibrational modes, only the out-of-plane bend ν3 was not observed as it forms an IR- and Raman-inactive local mode phonon.

Organisation(s)
Department of Mineralogy and Crystallography
External organisation(s)
University of Canterbury, Australian Centre for Neutron Scattering
Journal
The Journal of Physical Chemistry Part A: Molecules, Spectroscopy, Kinetics, Environment and General Theory
Volume
124
Pages
9244-9251
No. of pages
8
ISSN
1089-5639
DOI
https://doi.org/10.1021/acs.jpca.0c07589
Publication date
11-2020
Peer reviewed
Yes
Austrian Fields of Science 2012
105113 Crystallography, 105116 Mineralogy, 104026 Spectroscopy
Keywords
ASJC Scopus subject areas
Geochemistry and Petrology
Portal url
https://ucrisportal.univie.ac.at/en/publications/f995e2a1-3e11-41b6-be19-83848ff2dd9a